Bubble Templated Flexible Ceramic Nanofiber Aerogels with Cascaded Resonant Cavities for High-Temperature Noise Absorption

ACS Nano. 2022 Sep 27;16(9):13740-13749. doi: 10.1021/acsnano.2c06011. Epub 2022 Aug 11.

Abstract

Aviation noise pollution has become a significant public health problem, especially with the endless improvement of flight speed and loading capacity. Existing aviation noise absorbers have fatal defects of large weight, weak high-temperature stability, and difficulty to achieve both good low-frequency (<1000 Hz) and high-frequency (up to 6000 Hz) noise absorption simultaneously. Herein, we report a robust strategy to create flexible ceramic nanofiber aerogels with cascaded resonant cavities by the air bubbles-assisted freeze-casting technology. The stable hinged resonance cavity structures coassembled by flexible ceramic nanofibers, soft montmorillonite nanosheets, and silica sol glue endow the aerogels with temperature-invariant compressibility (from -196 to 1100 °C) and bendability. Moreover, the comprehensive advantages of cascaded resonance cavities and interconnected fibrous networks enable flexible ceramic nanofiber aerogels to have temperature-invariant full-frequency noise absorption performance (noise reduction coefficient up to 0.66 in 63-6300 Hz). The synthesis of this flexible ceramic nanofiber aerogel provides a versatile platform for the design of high-efficiency noise-absorbing material for various fields.

Keywords: cascade resonance; fiber aerogels; flexible ceramic nanofibers; noise absorption; temperature-invariant compressibility.