Impact of Electric Field Disorder on Broken-Symmetry States in Ultraclean Bilayer Graphene

Nano Lett. 2022 Sep 28;22(18):7378-7385. doi: 10.1021/acs.nanolett.2c02119. Epub 2022 Sep 16.

Abstract

Bilayer graphene (BLG) has multiple internal degrees of freedom and a constant density of states down to the charge neutrality point when trigonal warping is ignored. Consequently, it is susceptible to various competing ground states. However, a coherent experimental determination of the ground state has been challenging due to the interaction-disorder interplay. Here we present an extensive transport study in a series of dually gated freestanding BLG devices and identify the layer-antiferromagnet as the ground state with a continuous strength across all devices. This strength correlates with the width of the state in the electric field. We systematically identify electric-field disorder─spatial variations in the interlayer potential difference─as the main source responsible for the observations. Our results pinpoint for the first time the importance of electric-field disorder on spontaneous symmetry breaking in BLG and solve a long-standing debate on its ground state. The electric-field disorder should be universal to all 2D materials.

Keywords: bilayer graphene; broken-symmetry state; disorder; domain wall; ground state.