The Green Extraction of Blueberry By-Products: An Evaluation of the Bioactive Potential of the Anthocyanin/Polyphenol Fraction

Int J Mol Sci. 2024 Oct 14;25(20):11032. doi: 10.3390/ijms252011032.

Abstract

In the context of a circular economy, this study explores the valorization of blueberry pomace (BP) as a source of bioactive compounds using sustainable extraction methods. Microwave-assisted extraction (MAE) and microwave-assisted subcritical water extraction (MASWE) were employed to obtain two distinct fractions: MAE 1° and MASWE 2°. The first extract, MAE 1°, obtained at 80 °C, had a high total anthocyanin content (21.96 mgCya-3-glu/gextract), making it suitable as a natural pigment. Additionally, MAE 1° exhibited significant enzyme inhibition, particularly against α-amylase and β-glucosidase, suggesting potential anti-diabetic and anti-viral applications. The second extract, MASWE 2°, obtained at 150 °C, contained a higher total phenolic content (211.73 mgGAE/gextract) and demonstrated stronger antioxidant activity. MASWE 2° showed greater inhibition of acetylcholinesterase and tyrosinase, indicating its potential for use in Alzheimer's treatment, skincare, or as a food preservative. MASWE 2° exhibited cytotoxicity against HeLa cells and effectively mitigated H2O2-induced oxidative stress in HaCat cells, with MAE 1° showing similar but less pronounced effects. A tested formulation combining MAE 1° and MASWE 2° extracts in a 3:2 ratio effectively enhanced anthocyanin stability, demonstrating its potential as a heat-stable pigment. The extract characteristics were compared with a conventional method (MeOH-HCl in reflux condition), and the protocol's sustainability was assessed using several green metric tools, which provided insights into its environmental impact and efficiency.

Keywords: anthocyanins; bioactivity; blueberry pomace; green metrics; microwave-assisted extraction; polyphenols; subcritical water extraction.

MeSH terms

  • Anthocyanins* / chemistry
  • Anthocyanins* / isolation & purification
  • Anthocyanins* / pharmacology
  • Antioxidants* / chemistry
  • Antioxidants* / isolation & purification
  • Antioxidants* / pharmacology
  • Blueberry Plants* / chemistry
  • HeLa Cells
  • Humans
  • Microwaves
  • Monophenol Monooxygenase / antagonists & inhibitors
  • Monophenol Monooxygenase / metabolism
  • Plant Extracts* / chemistry
  • Plant Extracts* / pharmacology
  • Polyphenols* / chemistry
  • Polyphenols* / isolation & purification
  • Polyphenols* / pharmacology

Substances

  • Anthocyanins
  • Plant Extracts
  • Antioxidants
  • Polyphenols
  • Monophenol Monooxygenase

Grants and funding

The authors gratefully acknowledge the University of Turin for providing financial support (Ricerca Locale 2023).