Design, synthesis, biological evaluation, and X-ray single crystal structure of novel computer-aided-drug-designbased α-mangostin derivatives: Multifunctional ligands against Alzheimer's disease

Arch Pharm (Weinheim). 2025 Mar;358(3):e2400671. doi: 10.1002/ardp.202400671.

Abstract

Multifunctional ligand design strategy may be a promising approach for the treatment of Alzheimer's disease (AD). α-Mangostin (α-M), a natural small molecule with anti-AD properties, was used as the lead compound for the design and synthesis of six α-M derivatives (1-6) with the help of computer-aided-drug-design (CADD). Both theoretical calculations and experimental results suggested that 1-6 might serve as promising selective butyrylcholinesterase (BuChE) inhibitors and amyloid-β (Aβ) aggregation inhibitors. Meanwhile, experimental results confirmed the high selectivity of the derivatives, in which 1 had the best inhibitory activity and selectivity on BuChE (IC50 = 0.016 µM, SI = 700.63). The experimental results also showed that 1-6 could act as copper chelators and reactive oxygen species (ROS) scavengers. Furthermore, in vivo experiments with Caenorhabditis elegans also showed that 1 could scavenge ROS and inhibit Aβ aggregation. Notably, single crystals of 1, 4, and the 4-Cu(II) complex were prepared for the first time, which provided a reliable structural basis for analyzing the structure-activity relationship. The dimethylamino derivatives (1, 4) of α-M showed the best activities and were expected to become promising candidate drugs for multifunctional anti-AD.

Keywords: Alzheimer's disease; computer‐aided‐drug‐design; molecular dynamics; single crystal diffraction; α‐mangostin derivatives.

MeSH terms

  • Alzheimer Disease* / drug therapy
  • Amyloid beta-Peptides / antagonists & inhibitors
  • Amyloid beta-Peptides / metabolism
  • Animals
  • Butyrylcholinesterase / metabolism
  • Caenorhabditis elegans / drug effects
  • Chelating Agents / chemical synthesis
  • Chelating Agents / chemistry
  • Chelating Agents / pharmacology
  • Cholinesterase Inhibitors* / chemical synthesis
  • Cholinesterase Inhibitors* / chemistry
  • Cholinesterase Inhibitors* / pharmacology
  • Computer-Aided Design*
  • Copper / chemistry
  • Crystallography, X-Ray
  • Dose-Response Relationship, Drug
  • Drug Design*
  • Humans
  • Ligands
  • Molecular Structure
  • Reactive Oxygen Species / metabolism
  • Structure-Activity Relationship
  • Xanthones* / chemical synthesis
  • Xanthones* / chemistry
  • Xanthones* / pharmacology

Substances

  • Xanthones
  • mangostin
  • Amyloid beta-Peptides
  • Cholinesterase Inhibitors
  • Ligands
  • Butyrylcholinesterase
  • Reactive Oxygen Species
  • Copper
  • Chelating Agents