Point-of-Care Solid-Phase PCR in a Vertical Microfluidic Chip Integrated with All-Dielectric Nanostructured Metasurface for Highly Sensitive, Multiplexed Pathogen Detection

ACS Sens. 2025 Nov 28;10(11):8606-8615. doi: 10.1021/acssensors.5c02435. Epub 2025 Oct 19.

Abstract

Multiplexed solid-phase polymerase chain reaction (SP-PCR) has emerged as an indispensable modality for concurrent amplification of multiple genetic loci within a singular reaction vessel, facilitating efficient molecular diagnostics. Nevertheless, SP-PCR has seldom been integrated into point-of-care diagnostic devices due to several technical challenges, such as bubble formation during PCR, long reaction time, and low fluorescence signals generated from the PCR products on a solid surface. To circumvent these constraints, we engineered a microfluidic chip comprising SP-PCR and nanophotonic enhancement to enable highly sensitive, high-throughput, and cost-efficient molecular diagnostics. The chip's vertical orientation integrates preloaded reagent chambers for sequential lysis, washing, elution, and amplification, driven by a synchronized stepper motor and air vacuum, achieving robust nucleic acid purification and reverse transcription-PCR, and enabling bubble-free, gravity-assisted fluid dynamics during the PCR thermocycling. Thermal cycling is expedited through a dual-heater configuration alternating at subsecond intervals, obviating active cooling and shortening the reaction time. All-dielectric nanostructured metasurface was incorporated beneath the PCR chamber, allowing for the facile immobilization of DNA arrays to conduct SP-PCR. Taking advantage of guided-mode resonance supported by the metasurface and the SP-PCR approaches permits multiplexed detection and achieves a detection limit of 10 copies/reaction, highlighting the platform's potential for point-of-care diagnostics, personalized medicine, and high-throughput pathogen surveillance. Facile fabrication and automation emphasize scalability for mass production and deployment and collectively represent an advancement in point-of-care diagnostics.

Keywords: dielectric nanostructure; fluid manipulation; multiplexed detection; solid-phase PCR; vertical microfluidic.

MeSH terms

  • DNA, Bacterial / analysis
  • DNA, Bacterial / genetics
  • Humans
  • Lab-On-A-Chip Devices*
  • Limit of Detection
  • Microfluidic Analytical Techniques* / instrumentation
  • Multiplex Polymerase Chain Reaction* / instrumentation
  • Multiplex Polymerase Chain Reaction* / methods
  • Nanostructures* / chemistry
  • Point-of-Care Systems*

Substances

  • DNA, Bacterial