Total Synthesis of Okeaniamide A

Org Lett. 2026 Feb 13;28(6):2126-2130. doi: 10.1021/acs.orglett.5c05432. Epub 2026 Jan 23.

Abstract

The stereoselective total synthesis of okeaniamide A, a marine lipopeptide with therapeutic potential against diabetes mellitus and obesity, has been disclosed for the first time. The salient synthetic features include Negishi reaction, Kumada coupling, Julia-Kocienski olefination, and Crimmins acetate aldol reaction. Extension of the polyketide segment to the full molecular framework was achieved through consecutive peptide coupling, followed by late-stage oxidation at position C2. Okeaniamide A was found to be sensitive to C3 epimerization, particularly under oxidative and mildly acidic conditions.

MeSH terms

  • Depsipeptides* / chemical synthesis
  • Depsipeptides* / chemistry
  • Lipopeptides* / chemical synthesis
  • Lipopeptides* / chemistry
  • Molecular Structure
  • Oxidation-Reduction
  • Stereoisomerism

Substances

  • Lipopeptides
  • Depsipeptides