Tumour acidosis remodels the glycocalyx to control lipid scavenging and ferroptosis

Nat Cell Biol. 2026 Mar;28(3):567-580. doi: 10.1038/s41556-026-01879-y. Epub 2026 Feb 11.

Abstract

Aggressive tumours are defined by microenvironmental stress adaptation and metabolic reprogramming. Within this niche, lipid droplet accumulation has emerged as a key strategy to buffer toxic lipids and suppress ferroptosis. Lipid droplet formation can occur via de novo lipogenesis or extracellular lipid-scavenging. However, how tumour cells coordinate these processes remains poorly understood. Here we identify a chondroitin sulfate (CS)-enriched glycocalyx as a hallmark of the acidic microenvironment in glioblastoma and central nervous system metastases. This CS-rich glycocalyx encapsulates tumour cells, limits lipid particle uptake and protects against lipid-induced ferroptosis. Mechanistically, we demonstrate that converging hypoxia-inducible factor and transforming growth factor beta signalling induces a glycan switch on syndecan-1-replacing heparan sulfate with CS-thereby impairing its lipid-scavenging function. Dual inhibition of CS biosynthesis and diacylglycerol O-acyltransferase-1, a critical enzyme in lipid droplet formation, triggers catastrophic lipid peroxidation and ferroptotic cell death. These findings define glycan remodelling as a core determinant of metabolic plasticity, positioning the dynamic glycocalyx as a master regulator of nutrient access, ferroptotic sensitivity and therapeutic vulnerability in cancer.

MeSH terms

  • Acidosis* / metabolism
  • Acidosis* / pathology
  • Animals
  • Cell Line, Tumor
  • Chondroitin Sulfates / metabolism
  • Ferroptosis*
  • Glioblastoma* / metabolism
  • Glioblastoma* / pathology
  • Glycocalyx* / metabolism
  • Glycocalyx* / pathology
  • Humans
  • Lipid Metabolism*
  • Lipid Peroxidation
  • Metabolic Reprogramming
  • Mice
  • Signal Transduction
  • Transforming Growth Factor beta / metabolism
  • Tumor Microenvironment

Substances

  • Chondroitin Sulfates
  • Transforming Growth Factor beta