Green extraction of polyphenols from Berberis vulgaris using NADES: process optimization and extract characterization

Food Chem. 2026 Jul 1:516:149315. doi: 10.1016/j.foodchem.2026.149315. Epub 2026 Apr 17.

Abstract

Berberis vulgaris is a valuable source of bioactive polyphenols known for their antioxidant and antimicrobial properties. In this study, a green extraction method using the choline chloride: lactic acid: water (ChCl:LA:H2O) natural deep eutectic solvent (NADES) was developed to recover polyphenolic compounds from Berberis fruits. Using a Box-Behnken design, the optimal extraction conditions were determined to be 65 °C, a 5% water content, and a 0.055 liquid-to-solid ratio. These conditions resulted in a total phenolic content of 98.51 mg GAE/g and a DPPH radical scavenging activity of 89.91%. The temperature of 60 °C is selected as the final extraction temperature for future studies to ensure thermal stability and minimize degradation. Throughout at 4 °C the extract remained stable, maintaining high TPC and DPPH over time. Furthermore, the extract reduced browning in fresh-cut apples, maintaining the visual appearance for seven days. Moreover, the extract exhibited strong antibacterial activity against Gram-positive and Gram-negative bacteria. Therefore, this study demonstrates that NADES-based solvents, a green approach, provide an efficient, sustainable, and thermally stable method for the extraction of bioactive compounds from Berberis fruits, appropriate for food preservation and biodegradable active packaging applications.

Keywords: Antimicrobial properties; Antioxidant activity; Berberis vulgaris fruit; Box-Behnken design; Natural deep eutectic solvents; Polyphenols; Recovery.

Publication types

  • Evaluation Study

MeSH terms

  • Anti-Bacterial Agents / chemistry
  • Anti-Bacterial Agents / isolation & purification
  • Anti-Bacterial Agents / pharmacology
  • Antioxidants / chemistry
  • Antioxidants / isolation & purification
  • Antioxidants / pharmacology
  • Berberis* / chemistry
  • Chemical Fractionation* / instrumentation
  • Chemical Fractionation* / methods
  • Deep Eutectic Solvents / chemistry
  • Fruit / chemistry
  • Gram-Negative Bacteria / drug effects
  • Green Chemistry Technology* / methods
  • Plant Extracts* / chemistry
  • Plant Extracts* / isolation & purification
  • Plant Extracts* / pharmacology
  • Polyphenols* / chemistry
  • Polyphenols* / isolation & purification
  • Polyphenols* / pharmacology

Substances

  • Polyphenols
  • Plant Extracts
  • Anti-Bacterial Agents
  • Antioxidants
  • Deep Eutectic Solvents