Cloning, purification, and characterization of beta-cystathionase from Escherichia coli

Biochemistry. 1982 Jun 22;21(13):3064-9. doi: 10.1021/bi00256a005.

Abstract

The Clarke-Carbon clone bank of hybrid plasmid Escherichia coli DNA has been screened for plasmids able to complement an E. coli strain deficient for the production of beta-cystathionase. Clone 4-14 had the ability to complement a deletion mutation at this locus and expressed higher levels of beta-cystathionase than the wild-type strain. The transfer of the plasmid carried by this clone to a strain that constitutively expresses all the enzymes of the methionine biosynthetic pathway results in 100-fold overproduction of beta-cystathionase as compared to wild-type levels. With use of this strain, an efficient three-step purification scheme is described that gives 90% pure enzyme in 54% yield with a specific activity of 215 IU/mg. This enzyme is characterized as to molecular weight (280 000), number of subunits (six), pyridoxal phosphate binding (5.7 mol of pyridoxal phosphate bound/mol of protein, Km of 0.005 mM), amino acid composition, substrate specificity, and kinetic properties.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acids / analysis
  • Cloning, Molecular*
  • Cystathionine / genetics
  • Escherichia coli / enzymology*
  • Homocysteine / genetics
  • Kinetics
  • Lyases / genetics*
  • Molecular Weight
  • Plasmids
  • Pyridoxal Phosphate / pharmacology

Substances

  • Amino Acids
  • Homocysteine
  • Cystathionine
  • Pyridoxal Phosphate
  • Lyases
  • cystathionine beta-lyase