Pharmacology of L-744,453, a novel nonpeptidyl endothelin antagonist

Life Sci. 1996;58(14):1149-57. doi: 10.1016/0024-3205(96)00073-2.

Abstract

L-744,453 ((+/-)3-[4-(1-carboxy-1-(3,4-methylenedioxyphenyl)methoxy)-3,5-diprop ylphenyl methyl]-3H-imidazo[4,5-c]pyridine) is an endothelin (ET) receptor antagonist from a new structural class, the dipropyl-alpha-phenoxyphenylacetic acid derivatives. L-744,453 competitively and reversibly inhibits [125I]-ET-1 binding to Chinese Hamster Ovary cells expressing cloned human ET receptors (K(i)s: hET(A)=4.3 nM; hET(B)=232 nM), and is selective for endothelin receptors compared to other peptide receptors. It is an antagonist of ET-1 stimulated phosphatidyl inositol hydrolysis in rat uterine slices (IC50=220 nM) and exhibits no agonist activity. This compound also inhibits ET-1 stimulated contraction of rat aortic rings with a K(b) value of 50 nM. L-744,453 protects against ET-1 induced lethality in mice after i.v. (AD50=13 mg/kg i.v.) or oral administration. This compound also antagonizes ET-1 induced increases in diastolic blood pressure in conscious normotensive rats (AD50=0.67 mg/kg i.v.) and anesthetized ferrets (AD50=1.6 mg/kg i.v.). L-744,453 is a potent, selective, orally active endothelin antagonist which may be useful in elucidating the role of endothelin in normal and pathophysiological states.

Publication types

  • Comparative Study

MeSH terms

  • Animals
  • Biological Availability
  • Blood Pressure / drug effects
  • CHO Cells / drug effects
  • CHO Cells / metabolism
  • Cricetinae
  • Dioxoles / metabolism
  • Dioxoles / pharmacology*
  • Dioxoles / toxicity
  • Dogs
  • Endothelin Receptor Antagonists*
  • Endothelins / antagonists & inhibitors
  • Endothelins / metabolism
  • Endothelins / pharmacology
  • Female
  • Ferrets
  • Humans
  • Hydrolysis
  • Imidazoles / metabolism
  • Imidazoles / pharmacology*
  • Imidazoles / toxicity
  • In Vitro Techniques
  • Iodine Radioisotopes
  • Kinetics
  • Male
  • Mice
  • Muscle Contraction / drug effects
  • Phosphatidylinositols / metabolism
  • Rats
  • Rats, Sprague-Dawley
  • Receptors, Endothelin / metabolism
  • Structure-Activity Relationship

Substances

  • Dioxoles
  • Endothelin Receptor Antagonists
  • Endothelins
  • Imidazoles
  • Iodine Radioisotopes
  • L 744453
  • Phosphatidylinositols
  • Receptors, Endothelin