An in vivo approach for the identification of acceptor sites for O-glycosyltransferases: motifs for the addition of O-GlcNAc in Dictyostelium discoideum

Biochemistry. 1997 Apr 1;36(13):4034-40. doi: 10.1021/bi9617825.

Abstract

To identify and analyze acceptor sequences for O-glycosylation, we have developed an in vivo system expressing short peptides as glutathione S-transferase fusion proteins in the eukaryotic host Dictyostelium discoideum. Using this approach, we show that a short peptide motif (PTVTPT), present in the D. discoideum cell-surface glycoprotein PsA, is sufficient as a signal for O-glycosylation, even when fused to a heterologous protein. Monosaccharide analysis and solid-phase protein sequencing showed that the modification is a single N-acetylglucosamine attached to threonine residues. This was further confirmed by electrospray-mass spectrometry. The O-linked glycosylation of both this peptide and authentic PsA presents the modB-dependent carbohydrate-specific epitope identified by the monoclonal antibody MUD50. Substitution of threonine by serine residues in this peptide also yields a glycosylated fusion protein which is modified with single N-acetylglucosamine residues, but not all of the serines are glycosylated.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetylglucosamine / metabolism*
  • Amino Acid Sequence
  • Animals
  • Antibodies, Monoclonal / immunology
  • Blotting, Western
  • Dictyostelium / metabolism*
  • Electrophoresis, Polyacrylamide Gel
  • Factor Xa / metabolism
  • Gene Expression Regulation
  • Glycosylation
  • Glycosyltransferases / metabolism*
  • Mass Spectrometry
  • Molecular Sequence Data
  • Monosaccharides / analysis
  • Peptides / chemistry
  • Peptides / genetics
  • Peptides / metabolism*
  • Recombinant Fusion Proteins / chemistry
  • Recombinant Fusion Proteins / metabolism
  • Sequence Analysis

Substances

  • Antibodies, Monoclonal
  • Monosaccharides
  • Peptides
  • Recombinant Fusion Proteins
  • Glycosyltransferases
  • Factor Xa
  • Acetylglucosamine