Novel enzyme-linked immunoassay to determine nanogram levels of pneumocandins in human plasma

J Clin Microbiol. 1998 May;36(5):1414-8. doi: 10.1128/JCM.36.5.1414-1418.1998.

Abstract

A binding enzyme-linked immunosorbent assay (ELISA) has been developed for measuring nanogram concentrations of semisynthetic pneumocandin antifungal agents in human plasma. Semisynthetic pneumocandin L-733,560 was conjugated to succinylated hemocyanin by water-soluble carbodiimide and was used as an immunogen to produce polyclonal antibodies in rabbits. Pneumocandins were used to directly coat the wells of a microtiter plate, and quantitation was achieved by using rabbit polyclonal antibodies to pneumocandin L-733,560 and goat anti-rabbit immunoglobulin G conjugated to either alkaline phosphatase or horseradish peroxidase. Maximum binding of L-733,560 and most related analogs to the wells of the microtiter plate was found to occur in the first 5 min of incubation at 4 degrees C. Once bound to the plate, these pneumocandins could not be removed from the plate, either by treatment with 4.0 to 6.0 M urea or by treatment with 4.0 to 6.0 M guanidine hydrochloride for 24 h at 4 degrees C. The binding ELISA is linear with drug concentration and can detect levels of L-733,560 as low as 5 ng/ml in human plasma. The assay is also useful for quantitating plasma levels of related semisynthetic pneumocandins including clinical candidate MK-0991.

MeSH terms

  • Animals
  • Anti-Bacterial Agents / blood*
  • Anti-Bacterial Agents / immunology
  • Anti-Bacterial Agents / pharmacokinetics
  • Antibodies / immunology
  • Antibody Specificity
  • Antifungal Agents / blood*
  • Antifungal Agents / immunology
  • Antifungal Agents / pharmacokinetics
  • Dose-Response Relationship, Immunologic
  • Echinocandins
  • Enzyme-Linked Immunosorbent Assay / methods*
  • Humans
  • Peptides*
  • Peptides, Cyclic / blood*
  • Peptides, Cyclic / immunology
  • Peptides, Cyclic / pharmacokinetics
  • Rabbits

Substances

  • Anti-Bacterial Agents
  • Antibodies
  • Antifungal Agents
  • Echinocandins
  • L 733560
  • Peptides
  • Peptides, Cyclic
  • pneumocandin B(0)