Crystal structure of recombinant soybean beta-amylase complexed with beta-cyclodextrin

J Biol Chem. 1998 Jul 31;273(31):19859-65. doi: 10.1074/jbc.273.31.19859.

Abstract

In order to study the interaction of soybean beta-amylase with substrate, we solved the crystal structure of beta-cyclodextrin-enzyme complex and compared it with that of alpha-cyclodextrin-enzyme complex. The enzyme was expressed in Escherichia coli at a high level as a soluble and catalytically active protein. The purified recombinant enzyme had properties nearly identical to those of native soybean beta-amylase and formed the same crystals as the native enzyme. The crystal structure of recombinant enzyme complexed with beta-cyclodextrin was refined at 2. 07-A resolution with a final crystallographic R value of 15.8% (Rfree = 21.1%). The root mean square deviation in the position of C-alpha atoms between this recombinant enzyme and the native enzyme was 0.22 A. These results indicate that the expression system established here is suitable for studying structure-function relationships of beta-amylase. The conformation of the bound beta-cyclodextrin takes an ellipsoid shape in contrast to the circular shape of the bound alpha-cyclodextrin. The cyclodextrins shared mainly two glucose binding sites, 3 and 4. The glucose residue 4 was slightly shifted from the maltose binding site. This suggests that the binding site of the cyclodextrins is important for its holding of a cleaved substrate, which enables the multiple attack mechanism of beta-amylase.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Binding Sites
  • Crystallography, X-Ray
  • Cyclodextrins / chemistry*
  • Escherichia coli / genetics
  • Gene Expression / genetics
  • Glucose / metabolism
  • Glycine max / enzymology*
  • Hydrogen Bonding
  • Models, Molecular
  • Molecular Conformation
  • Molecular Sequence Data
  • Plant Proteins / chemistry
  • Recombinant Proteins / chemistry
  • Structure-Activity Relationship
  • beta-Amylase / chemistry*
  • beta-Cyclodextrins*

Substances

  • Cyclodextrins
  • Plant Proteins
  • Recombinant Proteins
  • beta-Cyclodextrins
  • beta-Amylase
  • Glucose
  • betadex

Associated data

  • GENBANK/D50866
  • PDB/1BFN