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Selenium Nucleophilicity and Electrophilicity in the Intra- and Intermolecular S(N)2 Reactions of Selenenyl Sulfide Probes.
Madabeni A, Zeisel L, Thorn-Seshold O, Orian L. Madabeni A, et al. Chemistry. 2025 Feb 25;31(12):e202404580. doi: 10.1002/chem.202404580. Epub 2025 Feb 3. Chemistry. 2025. PMID: 39847043 Free PMC article.
Chalcogenide exchange reactions are an important class of bimolecular nucleophilic substitution reactions (S(N)2) involving sulfur and selenium species as nucleophile, central atom, and/or leaving group, which are fundamental throughout redox biology and metabolism. While …
Chalcogenide exchange reactions are an important class of bimolecular nucleophilic substitution reactions (S(N)2) involving sulfur and se …
Bicyclic Selenenyl Sulfides with Tuned Bioreductive Step Rates Reveal Constraints for Probes Targeting Thioredoxin Reductase.
Zeisel L, Weissenhorn LD, Scholzen KC, Madabeni A, Orian L, Arnér ESJ, Thorn-Seshold O. Zeisel L, et al. Angew Chem Int Ed Engl. 2025 Aug 25;64(35):e202508911. doi: 10.1002/anie.202508911. Epub 2025 Jul 16. Angew Chem Int Ed Engl. 2025. PMID: 40583823 Free PMC article.
We accessed these densely functionalised cis- or trans-fused 1,2-thiaselenanes on gram scale over 5 steps by using a regioselective key step that elaborates an unusual, differentially protected 2,2'-bis-aziridine intermediate through sequential one-pot chalcogen introduction and …
We accessed these densely functionalised cis- or trans-fused 1,2-thiaselenanes on gram scale over 5 steps by using a regioselective key step …
Pathways and substrate specificity of DMSP catabolism in marine bacteria of the Roseobacter clade.
Dickschat JS, Zell C, Brock NL. Dickschat JS, et al. Chembiochem. 2010 Feb 15;11(3):417-25. doi: 10.1002/cbic.200900668. Chembiochem. 2010. PMID: 20043308
In contrast, the dealkylation activity for diethylsulfoniopropionate was strongly reduced, resulting in only small amounts of EtSH-derived volatiles accompanied by diethyl sulfide in P. gallaeciensis and O. indolifex, while D. shibae produced the related oxidation product …
In contrast, the dealkylation activity for diethylsulfoniopropionate was strongly reduced, resulting in only small amounts of EtSH-derived v …
Isotopically labeled sulfur compounds and synthetic selenium and tellurium analogues to study sulfur metabolism in marine bacteria.
Brock NL, Citron CA, Zell C, Berger M, Wagner-Döbler I, Petersen J, Brinkhoff T, Simon M, Dickschat JS. Brock NL, et al. Beilstein J Org Chem. 2013 May 15;9:942-50. doi: 10.3762/bjoc.9.108. Print 2013. Beilstein J Org Chem. 2013. PMID: 23766810 Free PMC article.
Members of the marine Roseobacter clade can degrade dimethylsulfoniopropionate (DMSP) via competing pathways releasing either methanethiol (MeSH) or dimethyl sulfide (DMS). Deuterium-labeled [(2)H6]DMSP and the synthetic DMSP analogue dimethyltelluriopropionate (DMTeP) wer …
Members of the marine Roseobacter clade can degrade dimethylsulfoniopropionate (DMSP) via competing pathways releasing either methanethiol ( …
Altered toxicity of organic pollutants in water originated from simultaneous exposure to UV photolysis and CdSe/ZnS quantum dots.
Kušić H, Leszczynska D. Kušić H, et al. Chemosphere. 2012 Oct;89(7):900-6. doi: 10.1016/j.chemosphere.2012.05.017. Epub 2012 Jun 6. Chemosphere. 2012. PMID: 22677523
The consistent pattern of changes in measured toxicity (TU) was observed and correlated with degradation of phenol and/or toluene. Spearman rank coefficients (SRCs) for data pairs sum-parameters vs. TU were calculated. The highest correlation between toxicity and de …
The consistent pattern of changes in measured toxicity (TU) was observed and correlated with degradation of phenol and/or toluene. Sp …