Glycoconjugated Metallohelices have Improved Nuclear Delivery and Suppress Tumour Growth In Vivo

Angew Chem Int Ed Engl. 2020 Aug 17;59(34):14677-14685. doi: 10.1002/anie.202006814. Epub 2020 Jul 7.

Abstract

Monosaccharides are added to the hydrophilic face of a self-assembled asymmetric FeII metallohelix, using CuAAC chemistry. The sixteen resulting architectures are water-stable and optically pure, and exhibit improved antiproliferative selectivity against colon cancer cells (HCT116 p53+/+ ) with respect to the non-cancerous ARPE-19 cell line. While the most selective compound is a glucose-appended enantiomer, its cellular entry is not mainly glucose transporter-mediated. Glucose conjugation nevertheless increases nuclear delivery ca 2.5-fold, and a non-destructive interaction with DNA is indicated. Addition of the glucose units affects the binding orientation of the metallohelix to naked DNA, but does not substantially alter the overall affinity. In a mouse model, the glucose conjugated compound was far better tolerated, and tumour growth delays for the parent compound (2.6 d) were improved to 4.3 d; performance as good as cisplatin but with the advantage of no weight loss in the subjects.

Keywords: antitumor agents; glycoconjugates; metallohelices; nuclear delivery; self-assembly.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Glycoconjugates / chemistry*
  • HCT116 Cells
  • Humans
  • Metals / chemistry*
  • Neoplasms / pathology*
  • Proton Magnetic Resonance Spectroscopy
  • Spectrometry, Mass, Electrospray Ionization

Substances

  • Glycoconjugates
  • Metals