Manganese (II) induces chemical hypoxia by inhibiting HIF-prolyl hydroxylase: implication in manganese-induced pulmonary inflammation

Toxicol Appl Pharmacol. 2009 Mar 15;235(3):261-7. doi: 10.1016/j.taap.2009.01.003.

Abstract

Manganese (II), a transition metal, causes pulmonary inflammation upon environmental or occupational inhalation in excess. We investigated a potential molecular mechanism underlying manganese-induced pulmonary inflammation. Manganese (II) delayed HIF-1alpha protein disappearance, which occurred by inhibiting HIF-prolyl hydroxylase (HPH), the key enzyme for HIF-1alpha hydroxylation and subsequent von Hippel-Lindau(VHL)-dependent HIF-1alpha degradation. HPH inhibition by manganese (II) was neutralized significantly by elevated dose of iron. Consistent with this, the induction of cellular HIF-1alpha protein by manganese (II) was abolished by pretreatment with iron. Manganese (II) induced the HIF-1 target gene involved in pulmonary inflammation, vascular endothelial growth factor (VEGF), in lung carcinoma cell lines.The induction of VEGF was dependent on HIF-1. Manganese-induced VEGF promoted tube formation of HUVEC. Taken together, these data suggest that HIF-1 may be a potential mediator of manganese-induced pulmonary inflammation.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cell Hypoxia / drug effects
  • Cell Hypoxia / physiology
  • Cell Line, Tumor
  • Chlorides / toxicity*
  • Humans
  • Hypoxia-Inducible Factor 1, alpha Subunit / antagonists & inhibitors*
  • Hypoxia-Inducible Factor 1, alpha Subunit / metabolism
  • Inflammation Mediators / toxicity*
  • Manganese Compounds
  • Pneumonia / chemically induced*
  • Pneumonia / enzymology*
  • Pneumonia / pathology
  • Procollagen-Proline Dioxygenase / antagonists & inhibitors*
  • Procollagen-Proline Dioxygenase / metabolism
  • Vascular Endothelial Growth Factor A / metabolism

Substances

  • Chlorides
  • HIF1A protein, human
  • Hypoxia-Inducible Factor 1, alpha Subunit
  • Inflammation Mediators
  • Manganese Compounds
  • VEGFA protein, human
  • Vascular Endothelial Growth Factor A
  • Procollagen-Proline Dioxygenase
  • manganese chloride